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By Rudy J. Koopmans (Eds.)

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A) and (b) Far-UV CD spectra in water at 20° C. 3 mM. The fibril spectrum reveals a red-shifted negative band (centered at 224 nm, compared to 214 nm for ribbons), possibly arising from the superposition of a strong aromatic CD band on the classical b-sheet CD spectrum. (c) Fit of the theoretical model (solid line) for the self-assembly of peptides into single and double b-sheet tapes, to the measured concentration dependence of the mean residue ellipticity [] of the negative CD band at  = 214 nm.

Chiral recognition in bis-urea-based aggregates and organogels through cooperative interactions’’. Angew. Chem. Int. Ed. 40(3), 613–616 (2001). P. ‘‘Supramolecular structure of a high-modulus polyaromatic fiber (Kevlar 49)’’. J. Polym. Sci. Part B-Polym. Phys. 15(12), 2201–2211 (1977). , and Mutter, M. ‘‘Switch-peptides: Controlling self-assembly of amyloid beta-derived peptides in vitro by consecutive triggering of acyl migrations’’. J. Am. Chem. Soc. 127(34), 11888–11889 (2005). , and Kirkham, J.

CHAPTER 3 Nucleation and Co-Operativity in Supramolecular Polymers Paul van der Schoot Contents 1. Introduction 2. Nucleated Assembly 3. Kinetics of Nucleated Assembly 4. Co-Operativity and Nucleation 5. Coarse Graining Reversed 6. Summary and Outlook Acknowledgement References 45 51 55 61 66 70 72 72 1. INTRODUCTION Supramolecular polymers are polymeric objects that spontaneously arise in solutions or melts from one or more types of molecular building block that can range from the chemically simple to the very complex (Ciferri, 2005).

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